The effect of adding up to 4 mass% of strontium to Mg-5Al-3Ca alloys was investigated in terms of microstructural and mechanical properties. The major interdendritic intermetallic compounds of as-cast alloys changed from the Mg(2)Ca phase to a combination of the (Mg,Al)(2)Ca and Al(4)Sr phases. The morphology of the interdendritic alpha-Mg/Al(4)Sr eutectic phase also changed from a coarse lamellar structure at a low strontium concentration to a bulk-like ultrafine lamellar structure at a high strontium concentration (4 mass%). The creep resistance was improved by the addition of up to 2 mass% strontium but it was saturated at a higher strontium concentration. [doi:10.2320/matertrans.M2010387]