DC Field | Value | Language |
---|---|---|
dc.contributor.author | Dong Heon Nam | ko |
dc.contributor.author | Zhang, Jenny Z. | ko |
dc.contributor.author | Andrei, Virgil | ko |
dc.contributor.author | Kornienko, Nikolay | ko |
dc.contributor.author | Heidary, Nina | ko |
dc.contributor.author | Wagner, Andreas | ko |
dc.contributor.author | Nakanishi, Kenichi | ko |
dc.contributor.author | Sokol, Katarzyna P. | ko |
dc.contributor.author | Slater, Barnaby | ko |
dc.contributor.author | Zebger, Ingo | ko |
dc.contributor.author | Hofmann, Stephan | ko |
dc.contributor.author | Fontecilla-Camps, Juan C. | ko |
dc.contributor.author | Park, Chan Beum | ko |
dc.contributor.author | Reisner, Erwin | ko |
dc.date.accessioned | 2018-09-18T05:51:27Z | - |
dc.date.available | 2018-09-18T05:51:27Z | - |
dc.date.created | 2018-08-27 | - |
dc.date.created | 2018-08-27 | - |
dc.date.created | 2018-08-27 | - |
dc.date.issued | 2018-08 | - |
dc.identifier.citation | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.57, no.33, pp.10595 - 10599 | - |
dc.identifier.issn | 1433-7851 | - |
dc.identifier.uri | http://hdl.handle.net/10203/245402 | - |
dc.description.abstract | Hydrogenases (H(2)ases) are benchmark electrocatalysts for H-2 production, both in biology and (photo)catalysis invitro. We report the tailoring of a p-type Si photocathode for optimal loading and wiring of H(2)ase through the introduction of a hierarchical inverse opal (IO) TiO2 interlayer. This proton-reducing Si vertical bar IO-TiO2 vertical bar H(2)ase photocathode is capable of driving overall water splitting in combination with a photoanode. We demonstrate unassisted (bias-free) water splitting by wiring Si vertical bar IO-TiO2 vertical bar H(2)ase to a modified BiVO4 photoanode in a photoelectrochemical (PEC) cell during several hours of irradiation. Connecting the Si vertical bar IO-TiO2 vertical bar H(2)ase to a photosystemII (PSII) photoanode provides proof of concept for an engineered Z-scheme that replaces the non-complementary, natural light absorber photosystemI with a complementary abiotic silicon photocathode. | - |
dc.language | English | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.title | Solar Water Splitting with a Hydrogenase Integrated in Photoelectrochemical Tandem Cells | - |
dc.type | Article | - |
dc.identifier.wosid | 000440899000030 | - |
dc.identifier.scopusid | 2-s2.0-85050516404 | - |
dc.type.rims | ART | - |
dc.citation.volume | 57 | - |
dc.citation.issue | 33 | - |
dc.citation.beginningpage | 10595 | - |
dc.citation.endingpage | 10599 | - |
dc.citation.publicationname | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | - |
dc.identifier.doi | 10.1002/anie.201805027 | - |
dc.contributor.localauthor | Park, Chan Beum | - |
dc.contributor.nonIdAuthor | Dong Heon Nam | - |
dc.contributor.nonIdAuthor | Zhang, Jenny Z. | - |
dc.contributor.nonIdAuthor | Andrei, Virgil | - |
dc.contributor.nonIdAuthor | Kornienko, Nikolay | - |
dc.contributor.nonIdAuthor | Heidary, Nina | - |
dc.contributor.nonIdAuthor | Wagner, Andreas | - |
dc.contributor.nonIdAuthor | Nakanishi, Kenichi | - |
dc.contributor.nonIdAuthor | Sokol, Katarzyna P. | - |
dc.contributor.nonIdAuthor | Slater, Barnaby | - |
dc.contributor.nonIdAuthor | Zebger, Ingo | - |
dc.contributor.nonIdAuthor | Hofmann, Stephan | - |
dc.contributor.nonIdAuthor | Fontecilla-Camps, Juan C. | - |
dc.contributor.nonIdAuthor | Reisner, Erwin | - |
dc.description.isOpenAccess | Y | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordAuthor | hydrogenase | - |
dc.subject.keywordAuthor | photoelectrochemistry | - |
dc.subject.keywordAuthor | photosynthesis | - |
dc.subject.keywordAuthor | silicon | - |
dc.subject.keywordAuthor | water splitting | - |
dc.subject.keywordPlus | H-2 PRODUCTION | - |
dc.subject.keywordPlus | PHOTOSYSTEM-II | - |
dc.subject.keywordPlus | EVOLUTION | - |
dc.subject.keywordPlus | OXYGEN | - |
dc.subject.keywordPlus | CATALYST | - |
dc.subject.keywordPlus | PHOTOANODE | - |
dc.subject.keywordPlus | REDUCTION | - |
dc.subject.keywordPlus | CHEMISTRY | - |
dc.subject.keywordPlus | OXIDATION | - |
dc.subject.keywordPlus | EFFICIENT | - |
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