The Hydration Structure at Yttria-Stabilized Cubic Zirconia (110)-Water Interface with Sub-Angstrom Resolution

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dc.contributor.authorHou, Binyangko
dc.contributor.authorKim, Seunghyunko
dc.contributor.authorPark, Changyongko
dc.contributor.authorKim, Taehoko
dc.contributor.authorKim, Jongjinko
dc.contributor.authorHong, Daniel Seungbumko
dc.contributor.authorBahn, Chi Bumko
dc.contributor.authorKim, Ji Hyunko
dc.date.accessioned2016-11-30T01:26:24Z-
dc.date.available2016-11-30T01:26:24Z-
dc.date.created2016-11-08-
dc.date.created2016-11-08-
dc.date.created2016-11-08-
dc.date.created2016-11-08-
dc.date.issued2016-06-
dc.identifier.citationSCIENTIFIC REPORTS, v.6-
dc.identifier.issn2045-2322-
dc.identifier.urihttp://hdl.handle.net/10203/214139-
dc.description.abstractThe interfacial hydration structure of yttria-stabilized cubic zirconia (110) surface in contact with water was determined with similar to 0.5 angstrom resolution by high-resolution X-ray reflectivity measurement. The terminal layer shows a reduced electron density compared to the following substrate lattice layers, which indicates there are additional defects generated by metal depletion as well as intrinsic oxygen vacancies, both of which are apparently filled by water species. Above this top surface layer, two additional adsorbed layers are observed forming a characteristic interfacial hydration structure. The first adsorbed layer shows abnormally high density as pure water and likely includes metal species, whereas the second layer consists of pure water. The observed interfacial hydration structure seems responsible for local equilibration of the defective surface in water and eventually regulating the long-term degradation processes. The multitude of water interactions with the zirconia surface results in the complex but highly ordered interfacial structure constituting the reaction front-
dc.languageEnglish-
dc.publisherNATURE PUBLISHING GROUP-
dc.titleThe Hydration Structure at Yttria-Stabilized Cubic Zirconia (110)-Water Interface with Sub-Angstrom Resolution-
dc.typeArticle-
dc.identifier.wosid000384975800001-
dc.identifier.scopusid2-s2.0-84975045619-
dc.type.rimsART-
dc.citation.volume6-
dc.citation.publicationnameSCIENTIFIC REPORTS-
dc.identifier.doi10.1038/srep27916-
dc.contributor.localauthorHong, Daniel Seungbum-
dc.contributor.nonIdAuthorHou, Binyang-
dc.contributor.nonIdAuthorKim, Seunghyun-
dc.contributor.nonIdAuthorPark, Changyong-
dc.contributor.nonIdAuthorKim, Taeho-
dc.contributor.nonIdAuthorKim, Jongjin-
dc.contributor.nonIdAuthorBahn, Chi Bum-
dc.contributor.nonIdAuthorKim, Ji Hyun-
dc.description.isOpenAccessY-
dc.type.journalArticleArticle-
dc.subject.keywordPlusX-RAY REFLECTIVITY-
dc.subject.keywordPlusNEUTRON-SCATTERING-
dc.subject.keywordPlusHYDROTHERMAL DEGRADATION-
dc.subject.keywordPlusSURFACE-WATER-
dc.subject.keywordPlusZRO2-
dc.subject.keywordPlusADSORPTION-
dc.subject.keywordPlusDYNAMICS-
dc.subject.keywordPlusOXIDE-
dc.subject.keywordPlusNANOPARTICLES-
dc.subject.keywordPlusELECTROLYTE-
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