We propose and demonstrate a new method which employs time-of-flight detection of femtosecond laser pulses for precise height measurement of large steps. By using time-of-flight detection with fiber-loop optical-microwave phase detectors, precise measurement of large step height is realized. The proposed method shows uncertainties of 15 nm and 6.5 nm at sampling periods of 40 ms and 800 ms, respectively. This method employs only one free-running femtosecond mode-locked laser and requires no scanning of laser repetition rate, making it easier to operate. Precise measurements of 6 mu m and 0.5 mm step heights have been demonstrated, which show good functionality of this method for measurement of step heights. (c) 2018 Optical Society of America