DC Field | Value | Language |
---|---|---|
dc.contributor.author | Kumar, D. Praveen | ko |
dc.contributor.author | Rangappa, A. Putta | ko |
dc.contributor.author | Do, Khai H. | ko |
dc.contributor.author | Hong, Yul | ko |
dc.contributor.author | Gopannagari, Madhusudana | ko |
dc.contributor.author | Reddy, K. Arun Joshi | ko |
dc.contributor.author | Bhavani, P. | ko |
dc.contributor.author | Reddy, D. Amaranatha | ko |
dc.contributor.author | Kim, Tae Kyu | ko |
dc.date.accessioned | 2024-06-24T08:00:11Z | - |
dc.date.available | 2024-06-24T08:00:11Z | - |
dc.date.created | 2024-02-28 | - |
dc.date.issued | 2022-01 | - |
dc.identifier.citation | APPLIED SURFACE SCIENCE, v.572 | - |
dc.identifier.issn | 0169-4332 | - |
dc.identifier.uri | http://hdl.handle.net/10203/319996 | - |
dc.description.abstract | Two-dimensional (2D) organic semiconductors, such as graphitic carbon nitride (g-C3N4), have gained extensive attention as a green alternative and possible route for photocatalytic applications due to their appropriate bandgap for the effective utilization of the visible light region. This paper presents the development of few-layered 2D exfoliated g-C3N4 nanosheets (eCN) by exfoliating stacked g-C3N4 layers (CNs) followed by incorporating inorganic perovskite-based Ba2NbFeO6 (BNF) nanostructures for solar fuel production. The optimized BNF/eCN composite material showed a high rate of solar fuel production, such as H-2 production (1677 mu mol.h(-1).g(-1)), which is similar to 8-fold higher than simple g-C3N4 and CO2 conversion into CO (32 mu mol.h(-1).g(-1)) and CH4 (4.8 mu mol.h(-1).g(-1)) production, which is 2-fold higher than eCN. However, only CO production (5 mu mol.h(-1).g(-1)) was observed for the simple CN. The enhanced activity of composite material was due to the improved surface-active sites of g-C3N4 through exfoliation, the unique properties of BNF nanosheets, and their combination. The present BNF/eCN composite system showed the highest efficiency compared to earlier reported g-C3N4-based photocatalysts. | - |
dc.language | English | - |
dc.publisher | ELSEVIER | - |
dc.title | Noble metal free few-layered perovskite-based Ba2NbFeO6 nanostructures on exfoliated g-C3N4 layers as highly efficient catalysts for enhanced solar fuel production | - |
dc.type | Article | - |
dc.identifier.wosid | 000718386500004 | - |
dc.identifier.scopusid | 2-s2.0-85116059608 | - |
dc.type.rims | ART | - |
dc.citation.volume | 572 | - |
dc.citation.publicationname | APPLIED SURFACE SCIENCE | - |
dc.identifier.doi | 10.1016/j.apsusc.2021.151406 | - |
dc.contributor.localauthor | Kim, Tae Kyu | - |
dc.contributor.nonIdAuthor | Kumar, D. Praveen | - |
dc.contributor.nonIdAuthor | Rangappa, A. Putta | - |
dc.contributor.nonIdAuthor | Do, Khai H. | - |
dc.contributor.nonIdAuthor | Hong, Yul | - |
dc.contributor.nonIdAuthor | Gopannagari, Madhusudana | - |
dc.contributor.nonIdAuthor | Reddy, K. Arun Joshi | - |
dc.contributor.nonIdAuthor | Bhavani, P. | - |
dc.contributor.nonIdAuthor | Reddy, D. Amaranatha | - |
dc.description.isOpenAccess | N | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordAuthor | 2D materials | - |
dc.subject.keywordAuthor | Perovskite nanostructures | - |
dc.subject.keywordAuthor | Ba2NbFeO6 nanosheets | - |
dc.subject.keywordAuthor | g-C3N4 nanosheets | - |
dc.subject.keywordAuthor | photocatalytic H-2 production and CO2 conversion | - |
dc.subject.keywordAuthor | Exfoliation | - |
dc.subject.keywordPlus | GRAPHITIC CARBON NITRIDE | - |
dc.subject.keywordPlus | HYDROGEN-EVOLUTION | - |
dc.subject.keywordPlus | PHOTOCATALYTIC CONVERSION | - |
dc.subject.keywordPlus | FACILE SYNTHESIS | - |
dc.subject.keywordPlus | CDS NANORODS | - |
dc.subject.keywordPlus | NANOSHEETS | - |
dc.subject.keywordPlus | GRAPHENE | - |
dc.subject.keywordPlus | REDUCTION | - |
dc.subject.keywordPlus | CO2 | - |
dc.subject.keywordPlus | HETEROJUNCTION | - |
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