Water-Stable and Photo-Patternable Siloxane-Encapsulated Upconversion Nanoparticles toward Flexible Near-Infrared Phototransistors

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dc.contributor.authorLee, Injunko
dc.contributor.authorPark, Cheolminko
dc.contributor.authorKim, Tae Sooko
dc.contributor.authorKang, Minsooko
dc.contributor.authorOh, Hyeongyeolko
dc.contributor.authorJang, Jinhyeongko
dc.contributor.authorPark, Jungjaeko
dc.contributor.authorYuk, Jong Minko
dc.contributor.authorLee, Hohjaiko
dc.contributor.authorPark, Chan Beumko
dc.contributor.authorChoi, Sung-Yoolko
dc.contributor.authorKang, Kibumko
dc.contributor.authorLee, Wonryungko
dc.contributor.authorBae, Byeong-Sooko
dc.date.accessioned2023-06-29T08:01:01Z-
dc.date.available2023-06-29T08:01:01Z-
dc.date.created2023-04-10-
dc.date.issued2023-06-
dc.identifier.citationADVANCED OPTICAL MATERIALS, v.11, no.12-
dc.identifier.issn2195-1071-
dc.identifier.urihttp://hdl.handle.net/10203/310118-
dc.description.abstractUpconversion nanoparticles (UCNPs), as near-infrared (NIR) absorbers, are promising materials for use in flexible NIR photodetectors, which can be applied for wearable healthcare applications due to their advantages in a broad spectral range, high photostability, and biocompatibility. However, to apply UCNPs in wearable and large-area integrated devices, water stability and micro-patterning methods are required. In this work, the UCNPs are encapsulated with a siloxane polymer (UCNP@SiOx) via a sol-gel process to enable photo-patternability and photo-stabililty in water conditions. The UCNP@SiOx can be photo-patterned down to micron-scale feature sizes and exhibit no significant decrease in upconversion photoluminescence (PL) intensities and PL decay time after immersion in water for 2 h. Moreover, UCNP@SiOx is evaluated by an in vitro biocompatibility test and found to be non-toxic. By integrating the UCNP@SiOx with MoS2 phototransistors (MoS2 + UCNP@SiOx), the devices exhibit enhanced responsivity (0.79 A W-1) and specific detectivity (2.22 x 10(7) Jones), which are 2.8 times higher than in the bare MoS2 phototransistors, and excellent mechanical durability over 1000 cycles of 20% compression and re-stretch test. This work opens the way for the facile synthesis of water-stable and photo-patternable siloxane-encapsulated UCNPs and a strategy for fabricating high-performance flexible NIR phototransistors through wavelength conversion.-
dc.languageEnglish-
dc.publisherWILEY-V C H VERLAG GMBH-
dc.titleWater-Stable and Photo-Patternable Siloxane-Encapsulated Upconversion Nanoparticles toward Flexible Near-Infrared Phototransistors-
dc.typeArticle-
dc.identifier.wosid000955657000001-
dc.identifier.scopusid2-s2.0-85150651177-
dc.type.rimsART-
dc.citation.volume11-
dc.citation.issue12-
dc.citation.publicationnameADVANCED OPTICAL MATERIALS-
dc.identifier.doi10.1002/adom.202202469-
dc.contributor.localauthorYuk, Jong Min-
dc.contributor.localauthorPark, Chan Beum-
dc.contributor.localauthorChoi, Sung-Yool-
dc.contributor.localauthorKang, Kibum-
dc.contributor.localauthorBae, Byeong-Soo-
dc.contributor.nonIdAuthorKang, Minsoo-
dc.contributor.nonIdAuthorOh, Hyeongyeol-
dc.contributor.nonIdAuthorLee, Hohjai-
dc.contributor.nonIdAuthorLee, Wonryung-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordAuthorflexible electronics-
dc.subject.keywordAuthormolybdenum disulfide-
dc.subject.keywordAuthornear-infrared-
dc.subject.keywordAuthorphototransistors-
dc.subject.keywordAuthorsiloxane-
dc.subject.keywordAuthorsupconversion nanoparticle-
dc.subject.keywordPlusPHOTODETECTORS-
dc.subject.keywordPlusLUMINESCENCE-
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MS-Journal Papers(저널논문)EE-Journal Papers(저널논문)
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