DC Field | Value | Language |
---|---|---|
dc.contributor.author | Kim, Youngsik | ko |
dc.contributor.author | Choi, Hyekyoung | ko |
dc.contributor.author | Lee, Yeunhee | ko |
dc.contributor.author | Koh, Weon-kyu | ko |
dc.contributor.author | Cho, Eunhye | ko |
dc.contributor.author | Kim, Taewan | ko |
dc.contributor.author | Kim, Hamin | ko |
dc.contributor.author | Kim, Yong-Hyun | ko |
dc.contributor.author | Jeong, Hu Young | ko |
dc.contributor.author | Jeong, Sohee | ko |
dc.date.accessioned | 2021-09-08T07:50:15Z | - |
dc.date.available | 2021-09-08T07:50:15Z | - |
dc.date.created | 2021-09-08 | - |
dc.date.created | 2021-09-08 | - |
dc.date.created | 2021-09-08 | - |
dc.date.created | 2021-09-08 | - |
dc.date.issued | 2021-07 | - |
dc.identifier.citation | NATURE COMMUNICATIONS, v.12, no.1 | - |
dc.identifier.issn | 2041-1723 | - |
dc.identifier.uri | http://hdl.handle.net/10203/287675 | - |
dc.description.abstract | Despite the technological importance of colloidal covalent III-V nanocrystals with unique optoelectronic properties, their synthetic process still has challenges originating from the complex energy landscape of the reaction. Here, we present InP tetrapod nanocrystals as a crystalline late intermediate in the synthetic pathway that warrants controlled growth. We isolate tetrapod intermediate species with well-defined surfaces of (110) and ((1) over bar(1) over bar(1) over bar) via the suppression of further growth. An additional precursor supply at low temperature induces [(1) over bar(1) over bar(1) over bar]-specific growth, whereas the [110]-directional growth occurs over the activation barrier of 65.7 kJ/mol at a higher temperature, thus finalizes into the (111)-faceted tetrahedron nanocrystals. We address the use of late intermediates with well-defined facets at the sub-10 nm scale for the tailored growth of covalent III-V nanocrystals and highlight the potential for the directed approach of nanocrystal synthesis. | - |
dc.language | English | - |
dc.publisher | NATURE PORTFOLIO | - |
dc.title | Tailored growth of single-crystalline InP tetrapods | - |
dc.type | Article | - |
dc.identifier.wosid | 000686581300023 | - |
dc.identifier.scopusid | 2-s2.0-85111111329 | - |
dc.type.rims | ART | - |
dc.citation.volume | 12 | - |
dc.citation.issue | 1 | - |
dc.citation.publicationname | NATURE COMMUNICATIONS | - |
dc.identifier.doi | 10.1038/s41467-021-24765-7 | - |
dc.contributor.localauthor | Kim, Yong-Hyun | - |
dc.contributor.nonIdAuthor | Kim, Youngsik | - |
dc.contributor.nonIdAuthor | Choi, Hyekyoung | - |
dc.contributor.nonIdAuthor | Koh, Weon-kyu | - |
dc.contributor.nonIdAuthor | Cho, Eunhye | - |
dc.contributor.nonIdAuthor | Kim, Taewan | - |
dc.contributor.nonIdAuthor | Kim, Hamin | - |
dc.contributor.nonIdAuthor | Jeong, Hu Young | - |
dc.contributor.nonIdAuthor | Jeong, Sohee | - |
dc.description.isOpenAccess | Y | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordPlus | TOTAL-ENERGY CALCULATIONS | - |
dc.subject.keywordPlus | COLLOIDAL QUANTUM DOTS | - |
dc.subject.keywordPlus | SEMICONDUCTOR NANOCRYSTALS | - |
dc.subject.keywordPlus | ELECTRONIC-STRUCTURE | - |
dc.subject.keywordPlus | HIGHLY EFFICIENT | - |
dc.subject.keywordPlus | TRANSITION | - |
dc.subject.keywordPlus | CHEMISTRY | - |
dc.subject.keywordPlus | LIGHT | - |
dc.subject.keywordPlus | SE | - |
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