DC Field | Value | Language |
---|---|---|
dc.contributor.author | Wang, Lina | ko |
dc.contributor.author | Zhao, Yu | ko |
dc.contributor.author | Thomas, Morgan L. | ko |
dc.contributor.author | Dutta, Arghya | ko |
dc.contributor.author | Byon, Hye Ryung | ko |
dc.date.accessioned | 2018-05-24T02:45:10Z | - |
dc.date.available | 2018-05-24T02:45:10Z | - |
dc.date.created | 2018-05-19 | - |
dc.date.created | 2018-05-19 | - |
dc.date.created | 2018-05-19 | - |
dc.date.issued | 2016-01 | - |
dc.identifier.citation | CHEMELECTROCHEM, v.3, no.1, pp.152 - 157 | - |
dc.identifier.issn | 2196-0216 | - |
dc.identifier.uri | http://hdl.handle.net/10203/242381 | - |
dc.description.abstract | Shuttling of soluble polysulfide species within electrodes is one of the most challenging issues in lithium-sulfur (Li-S) batteries. The resulting deposition of polysulfide species reduces the conductivity of the metallic Li electrode and the quantity of active material. Here, we demonstrate pronounced suppression of polysulfide shuttle using a sulfide-impermeable glass-ceramic membrane, which is employed as separator between the positive and negative electrodes. As a result, highly stable Li-S electrochemistry occurs in the sulfur-dissolving tetrahydrofuran catholyte solution, which provides good capacity retention and Coulombic efficiency for cycling. This demonstration holds promise for practical next-generation batteries with marked reversibility and the possibility to increase the energy density when equipped with a catholyte flow-through mode. | - |
dc.language | English | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.subject | RAY-ABSORPTION SPECTROSCOPY | - |
dc.subject | ELECTRICAL ENERGY-STORAGE | - |
dc.subject | AQUEOUS CATHODE | - |
dc.subject | REDOX COUPLES | - |
dc.subject | FLOW BATTERY | - |
dc.subject | LITHIUM | - |
dc.subject | ELECTROLYTE | - |
dc.subject | DISCHARGE | - |
dc.subject | POLYSULFIDES | - |
dc.subject | SPECIATION | - |
dc.title | Sulfur-Based Catholyte Solution with a Glass-Ceramic Membrane for Li-S Batteries | - |
dc.type | Article | - |
dc.identifier.wosid | 000371253500020 | - |
dc.identifier.scopusid | 2-s2.0-84954362681 | - |
dc.type.rims | ART | - |
dc.citation.volume | 3 | - |
dc.citation.issue | 1 | - |
dc.citation.beginningpage | 152 | - |
dc.citation.endingpage | 157 | - |
dc.citation.publicationname | CHEMELECTROCHEM | - |
dc.identifier.doi | 10.1002/celc.201500342 | - |
dc.contributor.localauthor | Byon, Hye Ryung | - |
dc.contributor.nonIdAuthor | Wang, Lina | - |
dc.contributor.nonIdAuthor | Zhao, Yu | - |
dc.contributor.nonIdAuthor | Thomas, Morgan L. | - |
dc.contributor.nonIdAuthor | Dutta, Arghya | - |
dc.description.isOpenAccess | N | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordAuthor | catholytes | - |
dc.subject.keywordAuthor | energy storage | - |
dc.subject.keywordAuthor | lithium-sulfur batteries | - |
dc.subject.keywordAuthor | membranes | - |
dc.subject.keywordAuthor | shuttles | - |
dc.subject.keywordPlus | RAY-ABSORPTION SPECTROSCOPY | - |
dc.subject.keywordPlus | ELECTRICAL ENERGY-STORAGE | - |
dc.subject.keywordPlus | AQUEOUS CATHODE | - |
dc.subject.keywordPlus | REDOX COUPLES | - |
dc.subject.keywordPlus | FLOW BATTERY | - |
dc.subject.keywordPlus | LITHIUM | - |
dc.subject.keywordPlus | ELECTROLYTE | - |
dc.subject.keywordPlus | DISCHARGE | - |
dc.subject.keywordPlus | POLYSULFIDES | - |
dc.subject.keywordPlus | SPECIATION | - |
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