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College of Engineering(공과대학)Graduate school of EEWS(EEWS대학원)EEW-Journal Papers(저널논문)

Bottom-up synthesis of fully sp(2) hybridized three-dimensional microporous graphitic frameworks as metal-free catalysts

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dc.contributor.authorTalapaneni, Siddulu Naiduko
dc.contributor.authorKim, Jaehoonko
dc.contributor.authorJe, Sang Hyunko
dc.contributor.authorBuyukcakir, Onurko
dc.contributor.authorOh, Jihunko
dc.contributor.authorCoskun, Aliko
dc.date.accessioned2017-07-18T05:43:19Z-
dc.date.available2017-07-18T05:43:19Z-
dc.date.created2017-06-28-
dc.date.created2017-06-28-
dc.date.created2017-06-28-
dc.date.created2017-06-28-
dc.date.issued2017-06-
dc.identifier.citationJOURNAL OF MATERIALS CHEMISTRY A, v.5, no.24, pp.12080 - 12085-
dc.identifier.issn2050-7488-
dc.identifier.urihttp://hdl.handle.net/10203/224792-
dc.description.abstractWe report on the bottom-up synthesis of a fully sp(2)-hybridized nitrogenated three-dimensional microporous graphitic framework (3D-MGF) starting from a highly preorganized, saddle-shaped tetraphenylene derivative under ionothermal reaction conditions. The 3D-MGF showed high stability and a surface area of 928 m(2) g(-1) along with a narrow pore size distribution. Our approach enabled template-free inclusion of the third dimension into the graphitic frameworks while retaining p-conjugation and conductivity, which was verified by their activity as metal-free electrocatalysts for the hydrogen evolution reaction.-
dc.languageEnglish-
dc.publisherROYAL SOC CHEMISTRY-
dc.subjectHYDROGEN EVOLUTION REACTION-
dc.subjectNITROGEN-DOPED GRAPHENE-
dc.subjectCARBON NITRIDE-
dc.subjectFREE ELECTROCATALYST-
dc.subjectNANOPOROUS GRAPHENE-
dc.subjectOXYGEN REDUCTION-
dc.subjectGENERATION-
dc.subjectELECTRODES-
dc.subjectNANOTUBES-
dc.subjectOXIDATION-
dc.titleBottom-up synthesis of fully sp(2) hybridized three-dimensional microporous graphitic frameworks as metal-free catalysts-
dc.typeArticle-
dc.identifier.wosid000403664800013-
dc.identifier.scopusid2-s2.0-85021633853-
dc.type.rimsART-
dc.citation.volume5-
dc.citation.issue24-
dc.citation.beginningpage12080-
dc.citation.endingpage12085-
dc.citation.publicationnameJOURNAL OF MATERIALS CHEMISTRY A-
dc.identifier.doi10.1039/c7ta02733h-
dc.contributor.localauthorOh, Jihun-
dc.contributor.localauthorCoskun, Ali-
dc.contributor.nonIdAuthorTalapaneni, Siddulu Naidu-
dc.contributor.nonIdAuthorBuyukcakir, Onur-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordPlusHYDROGEN EVOLUTION REACTION-
dc.subject.keywordPlusNITROGEN-DOPED GRAPHENE-
dc.subject.keywordPlusCARBON NITRIDE-
dc.subject.keywordPlusFREE ELECTROCATALYST-
dc.subject.keywordPlusNANOPOROUS GRAPHENE-
dc.subject.keywordPlusOXYGEN REDUCTION-
dc.subject.keywordPlusGENERATION-
dc.subject.keywordPlusELECTRODES-
dc.subject.keywordPlusNANOTUBES-
dc.subject.keywordPlusOXIDATION-
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EEW-Journal Papers(저널논문)
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