Concise Total Synthesis and Stereochemical Revision of all (-)-Trigonoliimines

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The concise and enantioselective total syntheses of (-)-trigonoliimines A, B, and C are described. Our unified strategy to all three natural products is based on asymmetric oxidation and reorganization of a single bistryptamine, a sequence of transformations with possible biogenetic relevance. We revise the absolute stereo chemistry of (-)-trigonoliimines A, B, and C.
Publisher
AMER CHEMICAL SOC
Issue Date
2011-07
Language
English
Article Type
Article
Citation

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, v.133, no.28, pp.10768 - 10771

ISSN
0002-7863
DOI
10.1021/ja204597k
URI
http://hdl.handle.net/10203/201398
Appears in Collection
CH-Journal Papers(저널논문)
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