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BODIPY-Thiophene Copolymers as p-Channel Semiconductors for Organic Thin-Film Transistors

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dc.contributor.authorUsta, Hakanko
dc.contributor.authorYilmaz, M. Denizko
dc.contributor.authorAvestro, Alyssa-Jenniferko
dc.contributor.authorBoudinet, Damienko
dc.contributor.authorDenti, Mitchellko
dc.contributor.authorZhao, Weiko
dc.contributor.authorStoddart, James Fraserko
dc.contributor.authorFacchetti, Antonioko
dc.date.accessioned2014-08-29T01:27:33Z-
dc.date.available2014-08-29T01:27:33Z-
dc.date.created2014-02-03-
dc.date.created2014-02-03-
dc.date.issued2013-08-
dc.identifier.citationADVANCED MATERIALS, v.25, no.31, pp.4327 - 4334-
dc.identifier.issn0935-9648-
dc.identifier.urihttp://hdl.handle.net/10203/188756-
dc.description.abstractThe synthesis and physicochemical properties of a new class of BODIPY-based donor-acceptor π-conjugated polymers are presented. Solution-processed top-gate/bottom-contact (TG-BC) thin-film transistors on flexible plastic substrates exhibit air-stable p-channel activities with charge carrier mobilities as high as 0.17 cm2/V·s and current on/off ratios of 105-106, the highest reported to date for a BODIPY-based semiconductor. The results shown here indicate a significant charge-transport improvement (>10000×) in BODIPY-based polymeric semiconductors, demonstrating its potential in future organic optoelectronic applications.-
dc.languageEnglish-
dc.publisherWILEY-V C H VERLAG GMBH-
dc.subjectFIELD-EFFECT TRANSISTORS-
dc.subjectHIGH-MOBILITY-
dc.subjectSOLAR-CELLS-
dc.subjectHIGH-PERFORMANCE-
dc.subjectCONJUGATED POLYMERS-
dc.subjectCHARGE-TRANSPORT-
dc.subjectBAND-GAP-
dc.subjectSPECTROSCOPIC PROPERTIES-
dc.subjectCOMPLEMENTARY CIRCUITS-
dc.subjectBUILDING-BLOCKS-
dc.titleBODIPY-Thiophene Copolymers as p-Channel Semiconductors for Organic Thin-Film Transistors-
dc.typeArticle-
dc.identifier.wosid000329198400010-
dc.identifier.scopusid2-s2.0-84882452835-
dc.type.rimsART-
dc.citation.volume25-
dc.citation.issue31-
dc.citation.beginningpage4327-
dc.citation.endingpage4334-
dc.citation.publicationnameADVANCED MATERIALS-
dc.identifier.doi10.1002/adma.201300318-
dc.embargo.liftdate9999-12-31-
dc.embargo.terms9999-12-31-
dc.contributor.nonIdAuthorUsta, Hakan-
dc.contributor.nonIdAuthorYilmaz, M. Deniz-
dc.contributor.nonIdAuthorAvestro, Alyssa-Jennifer-
dc.contributor.nonIdAuthorBoudinet, Damien-
dc.contributor.nonIdAuthorDenti, Mitchell-
dc.contributor.nonIdAuthorZhao, Wei-
dc.contributor.nonIdAuthorFacchetti, Antonio-
dc.type.journalArticleArticle-
dc.subject.keywordAuthorbodipy-
dc.subject.keywordAuthorpolymer-
dc.subject.keywordAuthororganic semiconductor-
dc.subject.keywordAuthortransistor-
dc.subject.keywordPlusFIELD-EFFECT TRANSISTORS-
dc.subject.keywordPlusHIGH-MOBILITY-
dc.subject.keywordPlusSOLAR-CELLS-
dc.subject.keywordPlusHIGH-PERFORMANCE-
dc.subject.keywordPlusCONJUGATED POLYMERS-
dc.subject.keywordPlusCHARGE-TRANSPORT-
dc.subject.keywordPlusBAND-GAP-
dc.subject.keywordPlusSPECTROSCOPIC PROPERTIES-
dc.subject.keywordPlusCOMPLEMENTARY CIRCUITS-
dc.subject.keywordPlusBUILDING-BLOCKS-
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