Femtosecond photoelectron imaging of pyridazine: S1 lifetime and Femtosecond photoelectron imaging of pyridazine: S1 lifetime and „3s„nÀ1…,3p„nÀ1…… Rydberg state energetics

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dc.contributor.authorMatsumoto, Yoshiteru-
dc.contributor.authorKim, Sang Kyu-
dc.contributor.authorSuzuki, Toshinori-
dc.date.accessioned2009-08-21T06:21:30Z-
dc.date.available2009-08-21T06:21:30Z-
dc.date.issued2003-
dc.identifier.citationJournal of Chemical Physics, Vol.119, No.1, pp.300-303en
dc.identifier.issn0021-9606-
dc.identifier.urihttp://hdl.handle.net/10203/10652-
dc.description.abstractThe first real-time study on pyridazine in the S1(n,p*) state is presented. The S1 state is found to dephase with a time constant of 323617 ps at its origin, and the electronic dephasing mechanism is attributed to the S1– S0 internal conversion. The S1 lifetime is found to decrease rather sharply as the internal energy increases. The 3s (n21) and 3p (n21) Rydberg states of pyridazine are clearly identified in angle- and energy-resolved photoelectron images obtained in the (1128) photoionization scheme, providing their respective term values of 5.6860.03 and 6.2860.04 eV.en
dc.description.sponsorshipScience and Technology of Japanen
dc.language.isoen_USen
dc.publisherAmerican Institute of Physicsen
dc.subjectphotoelectron imagingen
dc.subjectpyridazineen
dc.subjectRydberg stateen
dc.subjectFemtoseconden
dc.titleFemtosecond photoelectron imaging of pyridazine: S1 lifetime and Femtosecond photoelectron imaging of pyridazine: S1 lifetime and „3s„nÀ1…,3p„nÀ1…… Rydberg state energeticsen
dc.typeArticleen
dc.identifier.doi10.1063/1.1578062-
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