A Formal Total Synthesis of Dysiherbaine and Neodysiherbaine A

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A domino olefin metathesis reaction of 1-alkyl-3-(allyloxy)-7-oxabicyclo[2.2.1]hept-5-enes 7 produced the fused bis(oxacyclic) structure for dysiherbaine and neodysiherbaine A (i.e., 6b) with the complete control of the relative stereochemistry at the quaternary carbon center and the ring junction of the dysiherbaine core skeleton. A formal total synthesis of dysiherbaine and neodysiherbaine A was achieved from 6b.
Publisher
WILEY-V C H VERLAG GMBH
Issue Date
2012-08
Language
English
Article Type
Article
Keywords

STEREOCONTROLLED TOTAL-SYNTHESIS; DIELS-ALDER REACTION; AMINO-ACID; BIOLOGICAL EVALUATION; METATHESIS REACTIONS; KAINATE RECEPTORS; MARINE SPONGE; ANALOGS; (-)-DYSIHERBAINE; FURAN

Citation

EUROPEAN JOURNAL OF ORGANIC CHEMISTRY, no.22, pp.4192 - 4199

ISSN
1434-193X
DOI
10.1002/ejoc.201200439
URI
http://hdl.handle.net/10203/100634
Appears in Collection
CH-Journal Papers(저널논문)
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