Coherent transients mimicked by two-photon coherent control of a three-level system

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We show theoretically and experimentally that two-photon coherent control in a V-shape three-level system projects a one-photon coherent transient in a simple two-level system. The second-and third-order spectral phase terms of a shaped laser pulse play the roles of time and quadratic spectral phase, respectively, in conventional coherent transients. In a three-pulse coherent control experiment of atomic rubidium, the phase and amplitude of controlled transition probability is retrieved from a two-dimensional Fourier-transform spectral peak. It is hoped that this control scheme may harness coherent control capability on multidimensional Fourier-transform spectroscopy.
Publisher
AMER PHYSICAL SOC
Issue Date
2011-05
Language
English
Article Type
Article
Keywords

POPULATION TRANSFER; QUANTUM CONTROL; PULSES; SPECTROSCOPY; PHASE; EXCITATION; MOLECULES

Citation

PHYSICAL REVIEW A, v.83, no.5

ISSN
1050-2947
URI
http://hdl.handle.net/10203/99211
Appears in Collection
PH-Journal Papers(저널논문)
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