Catalytic enantioselective Mukaiyama-Michael reaction of 2-(trimethylsilyloxy)furan with alpha '-phenylsulfonyl enones

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The Mukaiyama-Michael reaction of 2-(trimethylsilyloxy)furan with alpha'-phenylsulfonyl enones using bis(oxazoline)copper(II) complexes as chiral catalyst provides the gamma-butenolides in high enantio- and diastereoselectivity. This approach is very useful for the enantioselective synthesis of gamma-butenolide derivatives under chiral Lewis acid catalysis.
Publisher
Georg Thieme Verlag Kg
Issue Date
2008-03
Language
English
Article Type
Article
Keywords

DIELS-ALDER REACTIONS; CHIRAL LEWIS-ACIDS; C(2)-SYMMETRIC COPPER(II) COMPLEXES; 4-SUBSTITUTED GAMMA-LACTONES; SILYL ENOL ETHERS; VINYL ETHERS; ALPHA,BETA-UNSATURATED KETONES; SILYLKETENE ACETALS; ADDITION-REACTION; ALDOL ADDITIONS

Citation

SYNLETT, no.4, pp.555 - 560

ISSN
0936-5214
DOI
10.1055/s-2008-1032074
URI
http://hdl.handle.net/10203/89589
Appears in Collection
CH-Journal Papers(저널논문)
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