Femtosecond photoelectron imaging of pyridazine: S-1 lifetime and (3s((n-1)), 3p((n-1))) Rydberg state energetics

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dc.contributor.authorMatsumoto, Yko
dc.contributor.authorKim, Sangkyuko
dc.contributor.authorSuzuki, Tko
dc.date.accessioned2013-03-04T03:18:18Z-
dc.date.available2013-03-04T03:18:18Z-
dc.date.created2012-02-06-
dc.date.created2012-02-06-
dc.date.issued2003-07-
dc.identifier.citationJOURNAL OF CHEMICAL PHYSICS, v.119, no.1, pp.300 - 303-
dc.identifier.issn0021-9606-
dc.identifier.urihttp://hdl.handle.net/10203/81707-
dc.description.abstractThe first real-time study on pyridazine in the S-1(n, pi*) state is presented. The S-1 state is found to dephase with a time constant of 323 +/- 17 ps at its origin, and the electronic dephasing mechanism is attributed to the S-1-S-0 internal conversion. The S-1 lifetime is found to decrease rather sharply as the internal energy increases. The 3s (n(-1)) and 3p (n(-1)) Rydberg states of pyridazine are clearly identified in angle- and energy-resolved photoelectron images obtained in the (1 + 2') photoionization scheme, providing their respective term values of 5.68 +/- 0.03 and 6.28 +/- 0.04 eV. (C) 2003 American Institute of Physics.-
dc.languageEnglish-
dc.publisherAMER INST PHYSICS-
dc.titleFemtosecond photoelectron imaging of pyridazine: S-1 lifetime and (3s((n-1)), 3p((n-1))) Rydberg state energetics-
dc.typeArticle-
dc.identifier.wosid000183585400035-
dc.identifier.scopusid2-s2.0-0038784521-
dc.type.rimsART-
dc.citation.volume119-
dc.citation.issue1-
dc.citation.beginningpage300-
dc.citation.endingpage303-
dc.citation.publicationnameJOURNAL OF CHEMICAL PHYSICS-
dc.identifier.doi10.1063/1.1578062-
dc.contributor.localauthorKim, Sangkyu-
dc.contributor.nonIdAuthorMatsumoto, Y-
dc.contributor.nonIdAuthorSuzuki, T-
dc.type.journalArticleArticle-
dc.subject.keywordPlusVIBRONIC LEVEL FLUORESCENCE-
dc.subject.keywordPlusELECTRONIC STATES-
dc.subject.keywordPlusPYRAZINE-
dc.subject.keywordPlusSPECTROSCOPY-
dc.subject.keywordPlusAZABENZENES-
dc.subject.keywordPlusRELAXATION-
dc.subject.keywordPlusMOLECULE-
dc.subject.keywordPlusSINGLET-
dc.subject.keywordPlusAZINES-
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