Total Synthesis of (−)-FD-838 and (−)-Cephalimysin A

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dc.contributor.authorJo, Deokheeko
dc.contributor.authorHan, Sunkyuko
dc.date.accessioned2019-08-06T00:20:03Z-
dc.date.available2019-08-06T00:20:03Z-
dc.date.created2019-08-05-
dc.date.created2019-08-05-
dc.date.issued2019-07-
dc.identifier.citationORGANIC LETTERS, v.21, no.15, pp.6045 - 6049-
dc.identifier.issn1523-7060-
dc.identifier.urihttp://hdl.handle.net/10203/264035-
dc.description.abstractWe completed a nine-step total synthesis of (−)-FD-838 and (−)-cephalimysin A. Our synthesis features a biogenetically guided assembly of the highly oxidized spirocyclic core by Snider-type tandem epoxidations of the chiral substrate derived from an amino acid derivative. Our synthetic approach provides a general and versatile solution to access spirocyclic PKS-NRPS-based secondary fungal metabolites.-
dc.languageEnglish-
dc.publisherAMER CHEMICAL SOC-
dc.titleTotal Synthesis of (−)-FD-838 and (−)-Cephalimysin A-
dc.typeArticle-
dc.identifier.wosid000480371600057-
dc.identifier.scopusid2-s2.0-85070895912-
dc.type.rimsART-
dc.citation.volume21-
dc.citation.issue15-
dc.citation.beginningpage6045-
dc.citation.endingpage6049-
dc.citation.publicationnameORGANIC LETTERS-
dc.identifier.doi10.1021/acs.orglett.9b02203-
dc.contributor.localauthorHan, Sunkyu-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordPlusABSOLUTE-CONFIGURATION-
dc.subject.keywordPlusMETABOLITE-
dc.subject.keywordPlusANGIOGENESIS-
dc.subject.keywordPlusPSEUROTIN-
dc.subject.keywordPlusPRODUCT-
dc.subject.keywordPlusFD-838-
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