High-yield production of few-layer boron nanosheets for efficient electrocatalytic N-2 reduction

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We report ambient electrochemical N-2 fixation at low overpotentials by using two-dimensional (2D) -boron. The metal-free catalyst afforded both an excellent NH3 yield rate and faradaic efficiency, approximately two times higher than those of bulk boron. We found that several binding sites, especially those involving icosahedral boron in the 2D material, can indeed catalyze N-2 reduction efficiently with strong N-2 adsorption, thus benefiting initial activation.
Publisher
ROYAL SOC CHEMISTRY
Issue Date
2019-04
Language
English
Article Type
Article
Citation

CHEMICAL COMMUNICATIONS, v.55, no.29, pp.4246 - 4249

ISSN
1359-7345
DOI
10.1039/c9cc00985j
URI
http://hdl.handle.net/10203/262411
Appears in Collection
EEW-Journal Papers(저널논문)
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