Expanding the Spectrum of Light-Driven Peroxygenase Reactions

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dc.contributor.authorWillot, Sebastien J. -P.ko
dc.contributor.authorFernandez-Fueyo, Elenako
dc.contributor.authorTieves, Florianko
dc.contributor.authorPesic, Miljako
dc.contributor.authorAlcalde, Miguelko
dc.contributor.authorArends, Isabel W. C. E.ko
dc.contributor.authorPark, Chan Beumko
dc.contributor.authorHollmann, Frankko
dc.date.accessioned2019-03-19T01:25:36Z-
dc.date.available2019-03-19T01:25:36Z-
dc.date.created2019-03-04-
dc.date.issued2019-02-
dc.identifier.citationACS CATALYSIS, v.9, no.2, pp.890 - 894-
dc.identifier.issn2155-5435-
dc.identifier.urihttp://hdl.handle.net/10203/251628-
dc.description.abstractPeroxygenases require a controlled supply of H2O2 to operate efficiently. Here, we propose a photocatalytic system for the reductive activation of ambient O-2 to produce H2O2 which uses the energy provided by visible light more efficiently based on the combination of wavelength-complementary photosensitizers. This approach was coupled to an enzymatic system to make formate available as a sacrificial electron donor. The scope and current limitations of this approach are reported and discussed.-
dc.languageEnglish-
dc.publisherAMER CHEMICAL SOC-
dc.titleExpanding the Spectrum of Light-Driven Peroxygenase Reactions-
dc.typeArticle-
dc.identifier.wosid000458707000012-
dc.identifier.scopusid2-s2.0-85060038413-
dc.type.rimsART-
dc.citation.volume9-
dc.citation.issue2-
dc.citation.beginningpage890-
dc.citation.endingpage894-
dc.citation.publicationnameACS CATALYSIS-
dc.identifier.doi10.1021/acscatal.8b03752-
dc.contributor.localauthorPark, Chan Beum-
dc.contributor.nonIdAuthorWillot, Sebastien J. -P.-
dc.contributor.nonIdAuthorFernandez-Fueyo, Elena-
dc.contributor.nonIdAuthorTieves, Florian-
dc.contributor.nonIdAuthorPesic, Milja-
dc.contributor.nonIdAuthorAlcalde, Miguel-
dc.contributor.nonIdAuthorArends, Isabel W. C. E.-
dc.contributor.nonIdAuthorHollmann, Frank-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordAuthorbiocatalysis-
dc.subject.keywordAuthorformate dehydrogenase-
dc.subject.keywordAuthorhydrogen peroxide formation-
dc.subject.keywordAuthoroxyfunctionalization-
dc.subject.keywordAuthorperoxygenases-
dc.subject.keywordAuthorphotocatalysis-
dc.subject.keywordPlusCATALYZED OXYFUNCTIONALIZATION-
dc.subject.keywordPlusOXIDATION-
dc.subject.keywordPlusPHOTOCHEMISTRY-
dc.subject.keywordPlusELECTRODE-
dc.subject.keywordPlusSYSTEM-
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