Photobiocatalysis: Activating Redox Enzymes by Direct or Indirect Transfer of Photoinduced Electrons

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dc.contributor.authorLee, Sahng Hako
dc.contributor.authorChoi, Da Somko
dc.contributor.authorKuk, Su Keunko
dc.contributor.authorPark, Chan Beumko
dc.date.accessioned2018-07-24T02:57:33Z-
dc.date.available2018-07-24T02:57:33Z-
dc.date.created2018-07-16-
dc.date.created2018-07-16-
dc.date.issued2018-07-
dc.identifier.citationANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.57, no.27, pp.7958 - 7985-
dc.identifier.issn1433-7851-
dc.identifier.urihttp://hdl.handle.net/10203/244534-
dc.description.abstractBiocatalytic transformation has received increasing attention in the green synthesis of chemicals because of the diversity of enzymes, their high catalytic activities and specificities, and mild reaction conditions. The idea of solar energy utilization in chemical synthesis through the combination of photocatalysis and biocatalysis provides an opportunity to make the "green" process greener. Oxidoreductases catalyze redox transformation of substrates by exchanging electrons at the enzymes active site, often with the aid of electron mediator(s) as a counterpart. Recent progress indicates that photoinduced electron transfer using organic (or inorganic) photosensitizers can activate a wide spectrum of redox enzymes to catalyze fuel-forming reactions (e.g., H-2 evolution, CO2 reduction) and synthetically useful reductions (e.g., asymmetric reduction, oxygenation, hydroxylation, epoxidation, Baeyer-Villiger oxidation). This Review provides an overview of recent advances in light-driven activation of redox enzymes through direct or indirect transfer of photoinduced electrons.-
dc.languageEnglish-
dc.publisherWILEY-V C H VERLAG GMBH-
dc.subjectSOLAR FUEL PRODUCTION-
dc.subjectPHOTOELECTROCHEMICAL BIOFUEL CELL-
dc.subjectARTIFICIAL PHOTOSYNTHESIS SYSTEM-
dc.subjectGRAPHITIC CARBON NITRIDE-
dc.subjectDRIVEN NADH REGENERATION-
dc.subjectGRAPHENE QUANTUM DOTS-
dc.subjectIRON-SULFUR CLUSTERS-
dc.subjectVISIBLE-LIGHT-
dc.subjectH-2 PRODUCTION-
dc.subjectCO2 REDUCTION-
dc.titlePhotobiocatalysis: Activating Redox Enzymes by Direct or Indirect Transfer of Photoinduced Electrons-
dc.typeArticle-
dc.identifier.wosid000436402100006-
dc.identifier.scopusid2-s2.0-85045090834-
dc.type.rimsART-
dc.citation.volume57-
dc.citation.issue27-
dc.citation.beginningpage7958-
dc.citation.endingpage7985-
dc.citation.publicationnameANGEWANDTE CHEMIE-INTERNATIONAL EDITION-
dc.identifier.doi10.1002/ange.201710070-
dc.contributor.localauthorPark, Chan Beum-
dc.contributor.nonIdAuthorLee, Sahng Ha-
dc.description.isOpenAccessN-
dc.type.journalArticleReview-
dc.subject.keywordAuthorartificial photosynthesis-
dc.subject.keywordAuthorelectron transfer-
dc.subject.keywordAuthorphotocatalysis-
dc.subject.keywordAuthorphotosensitizers-
dc.subject.keywordAuthorredox biocatalysis-
dc.subject.keywordPlusSOLAR FUEL PRODUCTION-
dc.subject.keywordPlusPHOTOELECTROCHEMICAL BIOFUEL CELL-
dc.subject.keywordPlusARTIFICIAL PHOTOSYNTHESIS SYSTEM-
dc.subject.keywordPlusGRAPHITIC CARBON NITRIDE-
dc.subject.keywordPlusDRIVEN NADH REGENERATION-
dc.subject.keywordPlusGRAPHENE QUANTUM DOTS-
dc.subject.keywordPlusIRON-SULFUR CLUSTERS-
dc.subject.keywordPlusVISIBLE-LIGHT-
dc.subject.keywordPlusH-2 PRODUCTION-
dc.subject.keywordPlusCO2 REDUCTION-
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