Programmable Electrochemical Rectifier Based on a Thin-Layer Cell

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A programmable electrochemical rectifier based on thin-layer electrochemistry is described here. Both the rectification ratio and the response time of the device are programmable by controlling the gap distance of the thin-layer electrochemical cell, which is easily controlled using commercially available beads. One of the electrodes was modified using a ferrocene-terminated self-assembled monolayer to offer unidirectional charge transfers via soluble redox species. The thin-layer configuration provided enhanced mass transport, which was determined by the gap thickness. The device with the smallest gap thickness (similar to 4 mu m) showed an unprecedented, high rectification ratio (up to 160) with a fast response time in a two-terminal configuration using conventional electronics.
Publisher
AMER CHEMICAL SOC
Issue Date
2017
Language
English
Article Type
Article
Citation

ACS APPLIED MATERIALS & INTERFACES, v.9, no.24, pp.20955 - 20962

ISSN
1944-8244
DOI
10.1021/acsami.7b02215
URI
http://hdl.handle.net/10203/225101
Appears in Collection
CH-Journal Papers(저널논문)
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