Sunlight-assisted, biocatalytic formate synthesis from CO2 and water using silicon-based photoelectrochemical cells

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We report on a silicon-based photoelectrochemical cell that integrates a formate dehydrogenase from Thiobacillus sp. (TsFDH) to convert CO2 to formate using water as an electron donor under visible light irradiation and an applied bias. Our current study suggests that the deliberate integration of biocatalysis to a light-harvesting platform could provide an opportunity to synthesize valuable chemicals with the use of earth abundant materials and sustainable resources
Publisher
ROYAL SOC CHEMISTRY
Issue Date
2016-08
Language
English
Article Type
Article
Keywords

ARTIFICIAL PHOTOSYNTHESIS; REDOX BIOCATALYSIS; NANOWIRES; EFFICIENCIES; POTENTIALS; CONVERSION; SYSTEM

Citation

CHEMICAL COMMUNICATIONS, v.52, no.62, pp.9723 - 9726

ISSN
1359-7345
DOI
10.1039/c6cc04661d
URI
http://hdl.handle.net/10203/213024
Appears in Collection
MS-Journal Papers(저널논문)
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